让下一篇重要论文，不再错过。

Large language models (LLMs) hold significant potential for psychological support, capable of generating empathetic responses and simulating therapeutic conversations. However, existing LLM-based approaches often lack sufficient grounding in structured diagnostic reasoning and diverse therapeutic strategies, limiting their effectiveness in complex counseling scenarios. To address these limitations, we propose PsyLLM, the first large language model designed to incorporate diagnostic- and therapeutic-oriented reasoning for mental health counseling. To develop PsyLLM, we design a novel automated data synthesis pipeline that processes real-world mental health posts collected from Reddit, where users frequently express psychological distress and seek community support. The pipeline transforms these posts into multi-turn counseling dialogues and leverages LLMs guided by international diagnostic standards (e.g., DSM/ICD) and multiple therapeutic frameworks (e.g., CBT, ACT, psychodynamic) to generate structured, clinically informed reasoning traces. A rigorous multi-dimensional filtering mechanism further improves the quality and clinical fidelity of the synthesized dialogue data. In addition, we introduce a new benchmark and evaluation protocol, assessing counseling performance across four key dimensions. Our experiments, along with evaluations by professional counseling experts, demonstrate that PsyLLM consistently outperforms various baseline models on this benchmark. Code, data, and models are available at https://github.com/Emo-gml/PsyLLM.